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Metastable magnetic phases in α-Dy2S3 induced by rotation of the single crystal in a magnetic field have been investigated. The compound α-Dy2S3 possesses an orthorhombic crystal structure having two crystallographically inequivalent Dy sites and shows successive antiferromagnetic transitions at TN1=11.4K and TN2=6.4K associated with various steep responses in physical properties. Anomalous enhancement...