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Peptides corresponding to the thrombin-binding loop of the fifth EGF-like domain of thrombomodulin (TM) extending from C407 to E426 (CECPEGYILDDGFICTDIDE) have been synthesized and their analysis has afforded an understanding of the structure and function of this region of TM. The results have implications for the design of thrombin inhibitors and give insight into the energetic factors that drive...