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Primary dynamics of photo-induced melting of charge order (CO) and metallic domain formation in [bis(ethlylenedithio)] tetrathiafulvalene (BEDT-TTF) salts α-(BEDT-TTF) 2 I 3 were studied using an infrared (1.4μm) pump–probe spectroscopy with a time resolution of 30fs. Faster (<30fs) and slower (ca. 2ps) responses of transient reflectivity accompanying the coherent phonon were detected...