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Two Cu(II) complexes of nitronyl-nitroxide-substituted pyrimidine (1) were prepared, and their structures and magnetic properties were clarified. The reaction of 1 with Cu(hfac) 2 gave a dark-green complex 2 with the formula [1 2 ·{Cu(hfac) 2 } 3 ], whereas the reaction with Cu(ClO 4 ) 2 in the presence of dien (diethylenetriamine) gave a dark-blue complex...
Magnetic interaction between two magnetic metals separated by a sizable diamagnetic ligand is generally very weak. A new spin-introduced bidentate, N-t-butyl-N-oxy-3,5-dipyridylaniline (1) was designed and synthesized to explore the spin-introducing effect on sizable ligands. A Mn(hfac) 2 complex of 1 was prepared and its structure was elucidated by X-ray structure analysis. The complex 1·Mn(hfac)...
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