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The ground state of Mn3C, a metastable but nonetheless fundamental phase in the context of high‐manganese steels, is still a matter of debate, and even the atomic structure of Mn3C has never been refined in the past. Moreover, Mn3C has been described as being nonmagnetic, antiferromagnetic, and also ferrimagnetic. Herein, Mn3C's crystal structure and its magnetic ground state were probed for the first...