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Achieving water splitting to produce green H2, using the noble‐metal‐free MoS2, has attracted huge interest from researchers. However, tuning the number of MoS2 layers precisely while obtaining small lateral sizes to surge the H2‐evolution rate is a tremendous challenge. Here, a bottom‐up strategy is designed for the in situ growth of ultrasmall lateral‐sized MoS2 with tunable layers on CdS nanorods...