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The titanium dioxide (TiO2) photocatalyst is only active under UV irradiation due to its wide‐gap nature. A novel excitation pathway denoted as interfacial charge transfer (IFCT) has been reported to activate copper(II) oxide nanoclusters‐loaded TiO2 powder (Cu(II)/TiO2) under visible‐light irradiation for only organic decomposition (downhill reaction) so far. Here, the photoelectrochemical study...