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Herein, a report on the growth of crystalline truncated pyramid microstructures by liquid‐phase epitaxy of Ga–As liquid phase on GaP (001) substrates under nonequilibrium (NEQ) conditions with different contact times and growth temperatures is provided. The micropyramids (MPs) have rectangular bases which are between 5 and 10 μm long, with the long sides aligned with the [110] direction. Remarkably,...