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Polylactic acid (PLA) composites having 1 wt% of MoS2 particles are prepared by solvent (SM) and melt mixing (MM) methods and their main thermal and mechanical properties are characterized. Coated films from SM samples and 3D‐printed filaments from MM samples are tested as active layers in reversible bilayer actuators using a paper sheet as a passive layer. The thermal properties depend on the method...