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This work is an attempt to understand the crystallization behavior of unconventional LAS (1:1.2:7) composition having MgO, BaO, K2O, and ZrO2. Crystallization parameters were determined using thermo‐analytical models based on differential scanning calorimetry (DSC). The activation energy of crystallization, E, and frequency factor, were calculated to be 354.40 kJ mol–1 K–1 and 1.63 × 1015, respectively...