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A lead‐free, completely inorganic, and nontoxic Cs2TiBr6‐based double perovskite solar cell (PSC) was simulated via SCAPS 1‐D. La‐doped BaSnO3 (LBSO) was applied as the electron transport layer (ETL) unprecedentedly in the simulation study of PSCs, while CuSbS2 was utilized as the hole transport layer (HTL). wxAMPS was used to validate the results of SCAPS simulations. Moreover, the first‐principle...