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Zeolitic Imidazolate Frameworks (ZIFs) are considered as a novel porous material combining high stability in inorganic zeolites with high porosity and organic functionality of MOFs. The cage‐like structure selectively and efficiently traps CO2, which is an indispensable and critical step for Electrocatalytic CO2 Reduction Reaction (CO2RR). In this work, ultrasmall ZIF‐8 nanomaterials are synthesized...