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The porous nano‐sized metal–organic framework (nanoMOF) and its proper surface modification could greatly promote the drug loading capability and introduce biocompatibility, biodegradability, and targeting functions into nano‐drug delivery systems. Herein, the HACD@ADA‐PA/MIL‐101_NH2 (Fe)‐P nanoparticle was successfully fabricated through supramolecular and coordination interactions from three building...