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2D magnets have recently drawn enormous interest. As an air‐stable A‐type van der Waals antiferromagnet (AFM), CrSBr has attracted great attention but has also led to controversies about its large‐span ordering temperatures. Herein, a systematic study of the magnetic phase transition in single‐crystalline CrSBr with ultrahigh‐quality through surface‐sensitive X‐ray magnetic linear dichroism and X‐ray...
The advent of van der Waals (vdW) ferromagnetic (FM) and antiferromagnetic (AFM) materials offers unprecedented opportunities for spintronics and magneto‐optic devices. Combining magnetic Kerr microscopy and density functional theory calculations, the AFM‐FM transition is investigated and a surprising abnormal magneto‐optic anisotropy in vdW CrSBr associated with different magnetic phases (FM, AFM,...
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