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Photocatalytic nitrogen reduction reaction (PNRR) is emerging as a sustainable ammonia synthesis approach to meet global carbon neutrality. Porous framework materials with well‐designed structures have great opportunities in PNRR; however, they suffer from unsatisfactory activity in the conventional gas‐in‐solvent system (GIS), owing to the hindrance of nitrogen utilization and strong competing hydrogen...
Electrochemical reduction of CO2 (CO2RR) and nitrogen (NRR) constitute alternatives to fossil fuel‐based technologies for the production of high‐value‐added chemicals. Yet their practical application is still hampered by the low energy and Faradaic efficiencies although numerous efforts have been paid to overcome the fatal shortcomings. To date, most studies have focused on designing and developing...
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