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A multifaceted Mo:BiVO4 (mf‐BVO) photoanode is grown on F‐doped‐SnO2 substrates via achemical bath deposition, and the crystal reconstruction process of mf‐BVO is found to boost the charge transport efficiency significantly for photoelectrochemical (PEC) water splitting. The mf‐BVO exhibits columnar grains with an uncommon (121) texture with high‐index facets such as (112), (020), (132), and (204)...