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The present paper deals with a “reactivity approach” to complex catalytic reactions. It utilizes data obtained with a reactor and demonstrates the very important role of both rate constants and concentrations of adsorbed species, on catalytic cycle, activity, and selectivity. It develops a link between global kinetics and closed sequence of elementary steps. It emphasizes the aspects of “assisted”...
Chemical kinetics makes it possible to discuss catalysis without chemistry. The general kinetic rules lead to generalities concerning catalytic mechanisms including rate constants, their impact on the turnover frequency of the cycle, product inhibition and catalyst development.
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