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A crystalline form of a glass-forming Ni-Nb-Zr-Ta alloy was studied as a hydrogen permeation membrane working in the temperature range from 573 K to 773 K. The crystalline membrane composed of an Nb-rich phase in an Ni10Zr7 matrix demonstrated a hydrogen permeation property superior to the membrane of the same chemical composition with an amorphous structure and the values of the hydrogen permeability...