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A novel multifunctional catalytic system has been developed for efficient hydrogen generation through the hydrolysis of ammonia borane. This system combines Pd NPs with acid sites and amines, which are both task-specific functionalities able to destabilize the N → B dative bond. The acidity of the support (zeolites of different structure and SiO2/Al2O3 ratio) used to disperse the Pd NPs causes an...