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Experiments designed to crystallize gas hydrate from dissolved CO 2 in natural porous media are used to study nucleation under varying thermodynamic conditions. We recover quantitative information from these experiments using a stochastic model for the nucleation process. Estimates of the model parameters are used to determine the average time for nucleation as a function of temperature and...
The solubility of CO 2 in liquid water inside the stability field of CO 2 -hydrate is determined experimentally. Equilibrium between liquid and hydrate phases is achieved in a porous medium to ensure that the stable phases are isolated from the vapor phase (which is used to maintain pressure). Changes in the solubility with temperature are monitored using measurements of electrical...
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