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A recent analysis of the enthalpy-driven swelling of a polymer brush by a compatible homopolymer leads to a simple swelling criterion that delineates the entropic and the enthalpic contributions. We consider the implications of this model for the formation of microphase in binary blends of a symmetric diblock copolymer (A-b-B) for which each block has a degree of polymerization (DP) = N and a homopolymer...
The formation of a microphase and a macrophase in solvent-cast homopolymer/block copolymer blends, where the homopolymer is exothermically miscible with one of the block copolymer segments, is demonstrated to depend on the molecular weights of the homopolymer and the incompatible segment of the block copolymer, in spite of the exothermic mixing. Binary blends of poly(vinyl chloride) (PVC) with poly(n-butyl...
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