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Single molecule spectroscopy experiments are reported for native peridinin–chlorophyll a–protein (PCP) complexes, and three reconstituted light-harvesting systems, where an N-terminal construct of native PCP from Amphidinium carterae has been reconstituted with chlorophyll (Chl) mixtures: with Chl a, with Chl b and with both Chl a and Chl b. Using laser excitation into peridinin (Per) absorption band...
We report on persistent spectral hole-burning studies of thiazine and oxazine dyes encapsulated in an AlPO 4 -5 aluminophosphate molecular sieve. A non-photochemical hole-burning mechanism is provided by small additional solvent molecules, e.g. glassy ethanol or amorphous water, in the pore system. Hole-burning efficiency and spontaneous hole-filling are in the typical range of glassy bulk...
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