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Direct synthesis (H2 + O2 → H2O2) could produce H2O2 (an environmentally benign oxidant) more cost-effectively and sustainably than anthraquinone oxidation, enabling broader use of H2O2 for industrial oxidations. We examine direct synthesis on AuxPd1 clusters to better understand the reasons for the high H2O2 selectivities of these materials. Steady-state H2O2 and H2O formation rates were measured...
Exogenously expressed opsins are valuable tools for optogenetic control of neurons in circuits. A deeper understanding of neural function can be gained by bringing control to endogenous neurotransmitter receptors that mediate synaptic transmission. Here we introduce a comprehensive optogenetic toolkit for controlling GABAA receptor-mediated inhibition in the brain. We developed a series of photoswitch ligands...
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