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The controlled formation of supramolecular architectures on chloride pre-covered Cu(100) has been studied by means of in situ scanning tunneling microscopy (STM) in an electrochemical environment. On top of the c(2×2)-Cl layer, ordered arrays of supramolecular cavitand structures could be obtained either by a surface assisted assembly of monomer building-blocks (1,1′-dibenzyl-4,4′-bipyridinium molecules)...
In situ electrochemical scanning tunneling microscopy has been used to examine the surface phase behavior of specifically adsorbed thiocyanate on Cu(100) within the potential range from −950 to −600 mV vs. Ag/AgSCN.In contact with the thiocyanate-containing electrolyte a highly ordered adsorbate layer is formed at negative potentials which can be described by a rectangular c(2×6)-4SCN unit-mesh corresponding...
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