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We present infrared and thermal desorption spectroscopic studies of CO adsorbed on size-selected nickel clusters composed of 11 atoms and supported on ultrathin magnesium oxide films. Thermal desorption spectroscopy of CO shows that on the average 4 molecules are weakly adsorbed per cluster at saturation coverage. Using an isotopic mixture of 12 CO and 13 CO, infrared spectroscopy...
Adsorption of Mn 2 (CO) 10 at 90 K on MgO(100) thin films grown onto Mo(100) has been investigated using thermal desorption spectroscopy and infrared reflection-absorption spectroscopy. The results of infrared spectroscopy are compared with gas-phase and solid-state studies of Mn 2 (CO) 10 . Heating a deposit of 3.5 monolayers to 800 K showed first molecular...
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