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In this work, atom probe field ion microscopy and transmission electron microscopy were used to study solute clustering, segregation and microstructure in two Al–Cu–Mg alloy systems, having different Cu:Mg ratios. The microstructural phases in a Ge modified Al–Cu–Mg alloy having a base composition in the α+θ field of the Al–Cu–Mg phase diagram exhibited an internal structure similar to a twinning...