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Surface structures of three zeolites, mordenite (MOR), heulandite (HEU), and Linde Type A (LTA), were investigated by using atomic force microscopy (AFM). The arrangement of 12-membered rings on the (001) surface of MOR was observed for the first time. Direct imaging of the morphological changes in the dissolving surface of HEU in an acidic or alkaline aqueous solution revealed that the aluminosilicate...