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Polymer electrolytes containing solvate ionic liquids (SILs) with increased toughness for use in lithium secondary batteries were designed by utilizing the self-assembly of ABA-type ionomer triblock copolymer, where the A-blocks are ionomers having strong intermolecular coulombic interactions. The ABA-type triblock copolymer, poly(lithium acrylate-r-acrylic acid)-b-poly(methyl methacrylate)-b-poly(lithium...