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The feasibility of direct laser cooling of silicon monofluoride (SiF) is investigated and assessed using the internally contracted multireference configuration interaction method with the Davidson correction and entirely uncontracted aug-cc-pwCV5Z basis sets. As for the A2Σ+(ν′=0)→X2Π transition, the computed radiative lifetime is 0.69μs and the vibrational branching ratio Rν′ν is highly diagonally...