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DC polarography is applied to study the effect of sucrose and glucose concentration in aqueous solutions on the rate of peroxodisulfate electroreduction. Non-monotonous dependence of reduction rate (current) on viscosity is found, which apparently contradicts the dependences expected for both diabatic and adiabatic reactions. The procedures of experimental data treatment are proposed, aimed to separation...
Some general and mutually intersecting problems of experimental studies and modeling the viscosity effects are considered in frames of the original study in sucrose and glucose aqueous solutions and reformulated in terms of the effect of non-Debye solvents. For the model reactants (Cr(III) and Co(III) complexes with ethylenediamminetetraacetate anion) the innresphere and solvent contributions to the...
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