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Hyperspectral goniometry reveals anisotropic scattering which dominates the visual appearance of self‐assembled polymer opals. The technique allows reconstruction of the reciprocal‐space of nanostructures, and indicates that chain defects formed during shear‐ordering are responsible for the anisotropy in these samples. Enhanced scattering with improving order is shown to arise from increased effective...
Permanent ordering of sub‐micrometer polymeric spheres by edge rotational shearing is reported. The resulting high‐quality, bulk, 3D‐ordered polymer opal thin‐films exhibit strikingly intense, tuneable structural color, which is applicable for photonics, metamaterials, nanoassembly, and structural color applications
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