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Two-dimensional (2D) infrared vibrational echoes were performed on horse heart carbonmonoxymyoglobin (MbCO) in water over a range of temperatures. The A1 and A3 conformational substates of MbCO are found to have different dephasing rates with different temperature dependences. A frequency–frequency correlation function derived from molecular dynamics simulations on MbCO at 298K is used to calculate...
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