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Computational studies of alicyclic silanediimines (RNSiNR) (rings five through twelve), mainly at the MP2/6-31G(d,p)//MP2/6-31G(d,p) level of theory, were conducted to (1) attempt to locate the transition states between silanediimines isomers, (2) follow their torsional IRC paths to either enantiomeric or diastereomeric pairs, and (3) compare silanediimine results with recently published, related...
Four silacyclobutyl anions have been prepared and studied by gas phase ion-molecule chemistry using newly modified tandem flowing afterglow instrumentation. These silacyclobutyl anions, which include a pentacoordinate adduct of 1,1-dimethylsilacyclobutane and fluoride and an α-silylcarbanion, siloxide, and mercaptide corresponding to 1,1-dimethylsilacyclobutane, have been characterized by their chemical...
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