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Densities of 3-methylpyridine (3-MP) + water and 3-methylpyridine + heavy water were measured in the 3-MP mole fraction range 0.002–0.04 from 298 to 318 K. The excess molar volumes of 3-MP + D2O mixtures were found to be more negative than those of 3-MP + H2O mixtures. The partial molar volume of 3-MP at infinite dilution is smaller in D2O than in H2O which suggests that 3-MP causes a structure-breaking...
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