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The high desorption temperature and slow kinetics still restrict the applications of LiAlH4 in hydrogen storage. To solve the above problems, NiTiO3@h‐BN and CoTiO3@h‐BN prepared for the first time are introduced into LiAlH4 by ball milling. LiAlH4 doped with 7 wt% NiTiO3@h‐BN, selected as an optimal doping sample, starts to release hydrogen at 68.1 °C, and the total amount of hydrogen released is...