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Synthesis of triangulene and its derivatives is challenging due to their intrinsic high spin nature. Herein, we report solution‐phase synthesis and isolation of a nitrogen‐doped triangulene (i.e., aza‐triangulene) (NT) and its cation (NT+) in single‐crystal form. Notably, the cation NT+ can be regarded as an isoelectronic structure of the corresponding all‐carbon triangulene. Both NT and NT+ show...
Synthesis of triangulene and its derivatives is challenging due to their intrinsic high spin nature. Herein, we report solution‐phase synthesis and isolation of a nitrogen‐doped triangulene (i.e., aza‐triangulene) (NT) and its cation (NT+) in single‐crystal form. Notably, the cation NT+ can be regarded as an isoelectronic structure of the corresponding all‐carbon triangulene. Both NT and NT+ show...
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