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The self‐assembly of N,N′,N″‐trialkylbenzene‐1,3,5‐tricarboxamides (BTAs) 1 or of “crowded” BTAs 11 and 12 lead to supramolecular columnar‐stacked structures with attractive material properties. The introduction of three alkoxy groups is reported to reinforce the self‐assembly process. The influence of a single substituent introduced onto the aromatic core of BTA significantly affects the self‐assembly...
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