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Generally, amine group captures CO2 according to 2:1 or 1:1 stoichiometry. Here, we report a kind of improved carbon capture using amino‐functionalized ionic liquids (ILs) through 1:2 stoichiometry. A serial of amino‐functionalized ILs various with basicity and steric hindrance of anion were designed, prepared, and applied in CO2 capture. Through a combination of absorption experiment, quantum chemical...
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