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Activity and selectivity of supported Ni, Pt, and Pd catalysts were studied in the liquidphase reductive amination of cyclohexanone at temperatures ranging from 100 to 150 °C. The catalyst 20% Ni/SiO2 is most active and selective providing a maximum yield of cyclohexylamine. The influence of the reaction conditions on the parameters of the catalytic process was studied. A detailed analysis of the...
Low-pressure on-stream conversion of cyclohexanone (CHN) was studied over HZSM-5 zeolites with various Si/Al ratios (different number of strong acid sites). Each conversion run was followed by thermal decomposition of surface species which also were investigated using FTIR spectroscopy. It was found that, below 300 o C, surface complexes consisting predominantly of CHN were held in the zeolites...
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