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The formic acid and methanol oxidation reaction are studied on Pt(111) modified by a pseudomorphic Pd monolayer (denoted hereafter as the Pt(111)–Pd 1ML system) in 0.1 M HClO 4 solution. The results are compared to the bare Pt(111) surface. The nature of adsorbed intermediates (CO ad ) and the electrocatalytic properties (the onset of CO 2 formation) were studied by...
The influence of various solvents upon the interfacial-potential profile on Pt(111) has been investigated by means of work-function changes and infrared frequency Stark shifts attending sequential-molecular dosing in ultra-high vacuum (UHV) at a suitably low temperature (ca. 100 K) with the primary objective of assessing the role of surface solvation in related electrochemical systems. The solvents...
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