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A series of crown ether‐based dinuclear bis(alkynyl)‐bridged gold(I) isocyanide complexes has been designed, synthesized, and characterized. The intramolecular Au···Au interactions of these complexes are used to bind potassium ions. Most of the bis(crown ether)‐containing gold(I) complexes are found to obey the 1:1 binding mode towards K+. Upon addition of K+ ions, the sandwich complex of crown ether...
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