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Pores are the most ubiquitous moieties in metal–organic frameworks (MOFs). Based on pore, the MOFs can thus communicate with various guest molecules, leading to many important applications such as storage, separation, and catalysis. However, its abundant surface, presenting another basic component, is often ignored. This is primarily due to the intrinsic stability of surface atoms of MOFs towards...
In their Concept article on page 13701 ff., F. Luo et al. present the MOF+ technique. The origin of this method is the surface reaction between Fe2+/or Fe3+ ions and phenol group in the metal–organic frameworks (MOFs), which is similar to the well‐known phenol‐Fe3+ reaction. Most importantly, this reaction only occurs on the surface of MOF samples, thus completely maintaining the pore and structure...
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