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Catalyst‐controlled functionalization of unmodified carbonyl compounds is a relevant operation in organic synthesis, especially when high levels of site‐ and stereoselectivity can be attained. This objective is now within reach for some subsets of enolizable substrates using various types of activation mechanisms. Recent contributions to this area include enantioselective transformations that proceed...
Extended enolates, particularly dienolates, may be generated upon deprotonation of α,β(and most usually β,γ)‐unsaturated carbonyl compounds by treatment with base. While known for more than half a century, their use in catalytic asymmetric bond‐forming reactions has remained underdeveloped until recently. The Minireview by M. Oiarbide and C. Palomo on page 10226 highlights the reactivity and selectivity...
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