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A major challenge in the pursuit of dynamic materials is the dichotomy between reversible structure and electronic conjugation. Guided by the precedence for N‐heterocyclic carbenes (NHCs) to dimerize, couple with electrophiles and bind to transition metals, we proposed that linearly opposed bis(NHC)s could, in a similar manner, afford unsaturated homopolymers, alternating copolymers, and metallopolymers...
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