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The cancer stem cell (CSC) toxicity and mechanism of action of a series of iridium(III) complexes bearing polypridyl and charged 1‐methyl‐2‐(2‐pyridyl)pyridinium ligands, 1–4 is reported. The most effective complex (containing 1,10‐phenanthroline), 3, kills CSCs and bulk cancer cells with equal potency (in the micromolar range), indicating that it could potentially remove heterogenous tumour populations...
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