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A triplet ground‐state diradical molecule, bis(nitronyl nitroxide)‐substituted diphenyldihydrophenazine (1..), that can be converted into a one‐electron oxidized species, 1…+, in the quartet ground state has been developed. Surprisingly, these species, 1.. and 1…+, can be used under ambient conditions because they are reasonably stable under aerobic conditions, even in solution. The temperature‐dependent...
The spin–spin and magnetic properties of two (nitronyl nitroxide)‐(di‐p‐anisylamine‐phenothiazine) diradical cation salts, (DAA‐PTZ)+‐NN⋅MBr4− (M=Ga, Fe), have been investigated. These diradical‐cation species were prepared by the cross‐coupling of iodophenothiazine DAA‐PTZ‐I with NN‐AuPPh3 followed by oxidation with the thianthrenium radical cation (TA+⋅MBr4−). These salts were found to be highly...
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