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The development of ordered graphene‐based materials combining high stability, large surface areas, ability to act as absorbent of relevant chemical species, and solution processability is of significance for energy applications. A poorly explored approach relies on the controlled nanostructuration of graphene into robust and highly ordered 3D networks as a route to further leverage the exceptional...
On page 1044, P. Samorì and co‐workers present the preparation of graphene‐based 3D covalent networks (G3DCNs) with tunable interlayer distances. The G3DCNs are prepared via controlled polymerization of benzidines with graphene oxide at different reaction temperatures under catalyst‐ and template‐free conditions. High‐performance supercapacitors are also achieved using the reduced form of G3DCNs as...
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