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While the synthesis of chloro formamidinium chloride has been known for over one century, no solid‐state structure of a chlorine‐substituted formamidinium compound has been reported up to now. Herein, we describe syntheses, solid‐state structures, and vibrational properties of four chloro formamidinium compounds, namely [ClC(NH2)2]Cl (1), [ClC(NH2)2](AuCl4) (2), [ClC(NH2)2]2(PdCl4) (3), and [ClC(NH...
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