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A zigzag‐type pore structure was proposed for the separation of a CO2/CH4 binary mixture by carbon molecular sieve membrane (CMSM). A defect‐free pore and three kinds of defect pores, i.e., random, uniform, and partial defect, were considered to improve the separation performance. Adsorption and diffusion behaviours of pure gases and a gas mixture were simulated by the grand canonical Monte Carlo...
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