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Treatment of the pentaphosphaferrocene [Cp*Fe(η5‐P5)] with CuI halides in the presence of different templates leads to novel fullerene‐like spherical molecules that serve as hosts for the templates. If ferrocene is used as the template the 80‐vertex ball [Cp2Fe]@[{Cp*Fe(η5‐P5)}12{CuCl}20] (4), with an overall icosahedral C80 topological symmetry, is obtained. This result shows the ability of ferrocene...
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